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Photocatalytic Decomposition of Liquid-Water On the Pt-Loaded TiO2 Catalysts: Effects of the Oxidation States of Pt Species On the Photocatalytic Reactivity and the Rate of the Back Reaction

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The photocatalytic decomposition of liquid water on Pt-loaded TiO2 (Pt/TiO2) catalysts was investigated. The results obtained by XPS and XRD measurements of the catalysts as a function of the calcination temperature as well as the photocatalytic decomposition reactions of H2O clearly indicate that controlling the oxidation state of Pt as well as the amount of loaded Pt species are both important factors in the design of water-splitting photocatalysts having high efficiency and stoichiometry.

Affiliations: 1: Department of Applied Chemistry, College of Engineering, Osaka Prefecture University, 1-1 Gakuencho, Sakai, Osaka 599-8531, JAPAN; 2: Research Institute of Innovative Technology for the Earth, Kizugawadai 9-2, Kizu-cho, Soraku-gun, Kyoto 619-0002, JAPAN


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