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Oxidative dehydrogenation of ethylbenzene with carbon dioxide over zeolite-supported iron oxide catalysts

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Oxidative dehydrogenation of ethylbenzene with carbon dioxide was carried out over ZSM-5 zeolite-supported iron oxide catalysts. In the presence of carbon dioxide, ethylbenzene was predominantly converted into styrene by oxidation. It was found that carbon dioxide in this reaction plays a role as a soft oxidant to greatly improve catalytic activity. An active phase for the dehydrogenation with carbon dioxide was suggested as rather reduced and isolated magnetite-like phase having oxygen deficiency in zeolite matrix.

10.1163/156856702760346879
/content/journals/10.1163/156856702760346879
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/content/journals/10.1163/156856702760346879
2017-08-22

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