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The reactions and composition of the surface intermediate species in the selective catalytic reduction of NOx with ethylene over Co-ZSM-5

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A pretreatment-transient reaction product analysis method was applied to study the reactions and average composition of the possible surface intermediate species in selective catalytic reduction with ethylene of NOx over Co-ZSM-5. The reactions of the surface species, formed by the pretreatment of Co-ZSM-5 in a NO/C2H4/O2 mixture at 275°C, with the NO/O2 flow produced much more N2 than that with the individual NO or O2 flow. The similarity of N2/COx/H2O product distribution generated from the above surface species-NO/O2 reactions and that from the normal NO/C2H4/O2 flow reactions implies that the surface species NCaObHc formed in the three-component pretreatment process is very likely the primary intermediate surface species generated during the real flow reactions. The in situ FT-IR (DRIFT) spectroscopy measurements of the surface species support the above conclusion.

Affiliations: 1: Laboratory of Plasma Physical Chemistry, Box 288, Dalian University of Technology, Dalian 116024, P. R. China

10.1163/156856707782565877
/content/journals/10.1163/156856707782565877
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/content/journals/10.1163/156856707782565877
2007-06-01
2017-02-23

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