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Organic crystals for second harmonic generation switching based on anil photochromes

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In photochromic materials, we demonstrated that non-linear optical (NLO) properties such as second harmonic generation (SHG) can be switched reversibly by alternate UV and visible irradiations. We report here on the design of materials fulfilling the prerequisites for SHG activity (push–pull and acentric space group) and photochromic properties. Photochromic and NLO properties of a series of anils are presented, along with the ability of some of them to switch SHG.

Affiliations: 1: Ecole Normale Supérieure de Cachan, Laboratoire de Photophysique et de Photochimie Supramoléculaires et Macromoléculaires (PPSM, CNRS UMR8531), Institut d'Alembert, 61 avenue du Président Wilson, 94235 Cachan Cedex, France; LASIR, USTL, 59655 Villeneuve d'Ascq Cedex, France; 2: Ecole Normale Supérieure de Cachan, Laboratoire de Photophysique et de Photochimie Supramoléculaires et Macromoléculaires (PPSM, CNRS UMR8531), Institut d'Alembert, 61 avenue du Président Wilson, 94235 Cachan Cedex, France; 3: Ecole Normale Supérieure de Cachan, Laboratoire de Photophysique et de Photochimie Supramoléculaires et Macromoléculaires (PPSM, CNRS UMR8531), Institut d'Alembert, 61 avenue du Président Wilson, 94235 Cachan Cedex, France; 4: Ecole Normale Supérieure de Cachan, Laboratoire de Photophysique et de Photochimie Supramoléculaires et Macromoléculaires (PPSM, CNRS UMR8531), Institut d'Alembert, 61 avenue du Président Wilson, 94235 Cachan Cedex, France; 5: Université Paris-Sud, Laboratoire de Chimie Inorganique, Institut de Chimie Moléculaire et des Matériaux d'Orsay (CNRS UMR8182), 91405 Orsay Cedex, France

10.1163/156856708783623447
/content/journals/10.1163/156856708783623447
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/content/journals/10.1163/156856708783623447
2008-02-01
2016-12-08

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