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CNT-based organic–inorganic composite materials with optoelectronic functionality

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This paper focuses on the fabrication of organic–inorganic composite materials with optoelectronic functionality based on carbon nanotubes (CNTs) by chemical and physical modifications. The one-dimensionally (1D) ordered composites of rare earth phthalocyanine compounds (RePc2) encapsulated by MWCNTs were obtained using a simple capillary filling method. The CNT-templated assembly of RePc2 nanowires was performed by a phase-separation method. Two other kinds of organic–inorganic 1D-ordered optoelectronic composites were prepared using the template method: coating MWCNTs with a fluorescent poly(triphenylamine) related co-polymer can be realized via a facile phase-separation strategy; 1D hybrid of bamboo-shaped CNTs covalently bound to RePc2. The relationship between the microstructure of the obtained 1D-ordered composites and optoelectronic properties was studied, and it was found that these ordered composites exhibited enhanced photoconductivity due to the charge transfer between the composite components.

Affiliations: 1: Department of Polymer Science and Engineering, State Key Lab of Silicon Materials, Zhejiang University, Hangzhou, 310027, P. R. China; Key Laboratory of Macromolecule Synthesis and Functionalization (Zhejiang University), Ministry of Education, Hangzhou 310027, P. R. China; 2: Department of Polymer Science and Engineering, State Key Lab of Silicon Materials, Zhejiang University, Hangzhou, 310027, P. R. China; Key Laboratory of Macromolecule Synthesis and Functionalization (Zhejiang University), Ministry of Education, Hangzhou 310027, P. R. China

10.1163/156856708783623528
/content/journals/10.1163/156856708783623528
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/content/journals/10.1163/156856708783623528
2008-02-01
2016-12-05

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