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Synthesis of one-dimensional microporous todorokite and its catalytic activity in CO oxidation

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Synthesis of an octahedral molecular sieve composed of Mn, Mg and O, known as todorokite, was studied in detail. The synthesis procedure is composed of three steps; layered birnessite synthesis, ion-exchange to buserite and final hydrothermal treatment of buserite. To obtain todorokites of different morphological properties, the aging time in the birnessite synthesis was varied. The effects of the aging time on properties of todorokites were studied by XRD, FE-SEM, TG-DTA, N2 adsorption–desorption, FT-IR and CO-TPD. In addition, catalytic activities of various todorokites for CO oxidation were investigated and the correlation between properties and activities was discussed.

Affiliations: 1: Department of Chemical Engineering, Faculty of Engineering, Kansai University, 3-3-35 Yamate-cho, Suita-shi 564-8680, Japan

10.1163/156856708784795527
/content/journals/10.1163/156856708784795527
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/content/journals/10.1163/156856708784795527
2008-05-01
2016-12-02

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