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A High-Power X-Band Pulsed Microwave Induced Catalytic Decomposition of Methane With Integral Acoustic Measurements

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A high-power microsecond pulsed microwave system operating in the X-band region was used for the catalytic conversion of methane. Microwave microsecond pulses at repetition rates of 50 and 80 Hz were used to initiate chemical reactions. The Microwave-Induced Acoustic technique was employed in combination with gas chromatography for on-line detection of chemical products. Methane was converted to C2 and C3 hydrocarbons. The selectivity of ethane in hydrocarbon products can be >90 %. The contribution of hydrogen evolution and carbon deposition has been shown to be important. A comparison between previous experiments performed with millisecond pulse durations is given.

Affiliations: 1: Department of Chemistry, Queens University, Kingston, CANADA K7L 3N6


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