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Electron-Transfer Photochemistry of 2,3-Diphenyl-1,3-Butadiene

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Photoinduced electron-transfer (ET) reaction of 2,3-diphenyl-1,3-butadiene 1 resulted in the formation of [4 + 2] dimer 8, [4 + 4] dimer 4, and its secondary product bicyclooctadiene 9. The ET induced dimerization of 1 is suggested to proceed through a stepwise mechanism involving a bis-allylic intermediate 10.

Affiliations: 1: Department of Chemistry, Faculty of Science, Tohoku University, Aoba-ku, Sendai 980-77, Japan


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