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Kinetics and Mechanism of One-Electron Oxidation of Bilirubin in Dichloromethane Solution

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Bilirubin (BR) was oxidized by tris-(4-bromophenyl)-ammonium hexachloroantimonate (1), 2,2,6,6-tetramethyl-4-acetyloxypiperidine oxoammonium hexachloroantimonate (2) and 2,2,6,6-tetramethyl-4-methoxypiperidine oxoamonium tetrafluoroborate (3) to the corresponding radical cation. The rate and activation parameters for the reaction were determined. An electron transfer mechanism is proposed based on the kinetic results.

Affiliations: 1: National Laboratory of Applied Organic Chemistry, Lanzhou University Lanzhou 730000, P.R. China; 2: Department of Modern Chemistry, University of Science and Technology of China, Hefei 230026, P.R. CHINA


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