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Photoinduced Electron Transfer Between C60 and N,N,N',N'-Tetramethylbenzidine (Ntmb). Fourier Transform Electron Paramagnetic Resonance Study

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Fourier transform EPR spectroscopy was employed in studying the electron transfer (ET) reaction and the quenching mechanisms of the photoexcited triplet state of C60 as electron acceptor and N,N,N',N'-tetramethylbenzidine (NTMB) as electron donor in benzonitrile solution. The ET reaction product, the cation radical NTMB•+, interacts with3*C60, leading to photoinduced electron polarization of NTMB•+ via triplet-doublet mixing mechanism combined with triplet mechanism. The quenching of 3*C60 and the polarization behavior of NTMB•+ are discussed.

Affiliations: 1: Department of Physical Chemistry and the Farkas Center for Light-Induced Processes, The Hebrew University of Jerusalem, Jerusalem 91904, Israel; 2: Institute of Molecular Physics, Free University of Berlin, 14195 Berlin, Germany


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