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The Design of Photocatalysts for the Removal of NOx At Normal Temperatures --Copper (I) and Silver (I) Ion Catalysts Anchored Within Zeolite Cavities

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The Cu+/ZSM-5 and Ag+/ZSM-5 catalysts were prepared by a combination of ion-exchange and thermovacuum treatments. In situ photoluminescence, ESR, XAFS, UV-VIS and FT-IR measurements of the catalysts revealed that within the cavity of the ZSM-5 zeolite, the Cu+ ion or Ag+ ion exists in an isolated state. UV irradiation of the catalysts in the presence of NO at normal temperature led to the formation of NZ and O2 for Cu+/ZSM-5 and N2, N2O and NO2 for Ag+/ZSM-5, indicating that the isolated Cu+ ion or Ag+ ion acts as a photocatalyst for the direct decomposition of NO. However, the Cu+/ZSM-5 catalyst loses its photocatalytic reactivity under the coexistence of O2, while the Ag+/ZSM-5 catalyst maintains its reactivity under the coexistence of O2 and H2O,

Affiliations: 1: Department of Applied Chemistry, College of Engineering, Osaka Prefecture University, Gakuen-cho 1-1, Sakai, Osaka 593, Japan

10.1163/156856797X00420
/content/journals/10.1163/156856797x00420
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/content/journals/10.1163/156856797x00420
1997-01-01
2016-12-04

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