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Oxide Nanoparticles Within a Host Microporous Matrix: Polynuclear Copper Species in Cu-Zm5 and Their Role in the Reduction of No

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The role of copper-oxide nanoparticles inside a host ZSM5 zeolite, identified by UV-Visible-NIR diffuse reflectance spectroscopy on the reactivity in NO reduction to N2 in the presence of propane/O2 or ammonia/O2 is discussed. These species lead to an enhancement in the rate of alkane depletion in the reduction of NO in the presence of propane/O2, whereas they cooperate with isolated ions at exchangeable sites in determining the overall catalytic behaviour in NO reduction in the presence of ammonia/O2. Also the stability of these species depends on the type of reductant.

Affiliations: 1: Dept. Industrial Chemistry, Univ. Messina, Salita Sperone 31, 98166 Messina, Italy, Dept. Ind. Chem. and Materials, V.le Risorgimento 4, 40136 Bologna, Italy; 2: Dept. Ind. Chem. and Materials, V.le Risorgimento 4, 40136 Bologna, Italy


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