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New Approaches To Free Radical Thermochemistry [11

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A variety of unusual techniques have been used to measure thermodynamic propeties of free radicals and heats of the reactions in which they participate. These include a radical buffer EPR technique, the appearance energy method, photoacoustic spectroscopy, and electrochemical detection of free radicals. The methods can be applied to systems involving organometallic and high molecular weight materials which are normally inaccessible to conventional, gas phase techniques.

Affiliations: 1: Division of Chemistry, National Research Council of Canada, Ottawa, Ontario, Canada, K1A 0R6


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